Moloi is a surname. Notable people with the surname include:
Dirang Moloi (born 1985), Botswanan footballer
Lerato Moloi, South African fashion model
Mpho Moloi (born 1983), South African footballer
Pontsho Moloi (born 1981), Botswanan footballer
Precious Moloi-Motsepe, South African fashion entrepreneur and philanthropist
Teboho Moloi (born 1968), South African footballer
Thabo Moloi (born 1994), South African footballer
Timothy Moloi (born 1975), South African singer
